Character Name : Gargamel

Original Name : Hank Azaria

Gender : Male

Character Name : Patrick Winslow

Original Name : Neil Patrick Harris

Gender : Male

Character Name : Grace Winslow

Original Name : Jayma Mays

Gender : Female

Character Name : Papa Smurf (voice)

Original Name : Jonathan Winters

Gender : Male

Character Name : Smurfette (voice)

Original Name : Katy Perry

Gender : Female

Character Name : Clumsy Smurf (voice)

Original Name : Anton Yelchin

Gender : Male

Character Name : Odile Anjelou

Original Name : Sofía Vergara

Gender : Female

Character Name : Henri

Original Name : Tim Gunn

Gender : Male

Character Name : Azrael (voice)

Original Name : Frank Welker

Gender : Male

Character Name : Model

Original Name : Madison McKinley

Gender : Female

Character Name : Model

Original Name : Meg Phillips

Gender : Male

Character Name : Cabbie

Original Name : Mahadeo Shivraj

Gender : Male

Character Name : Newscaster

Original Name : Julie Chang

Gender : Male

Character Name : Bluetooth Businessman

Original Name : Mark Doherty

Gender : Male

Character Name : Young Woman

Original Name : Minglie Chen

Gender : Female

Character Name : Guy in Plaid Shirt

Original Name : Sean Kenin

Gender : Male

Character Name : Bum

Original Name : Victor Pagan

Gender : Male

Character Name : Anjelou Employee

Original Name : Adria Baratta

Gender : Male

Character Name : Odile's Mother

Original Name : Paula Pizzi

Gender : Male

Character Name : Waiter

Original Name : Andrew Sellon

Gender : Male

Character Name : Little Sister

Original Name : Julianna Rigoglioso

Gender : Male

Character Name : Blonde Sister

Original Name : Daria Rae Figlo

Gender : Male

Character Name : Toy Salesperson

Original Name : Bradley Gosnell

Gender : Male

Character Name : Toy Store Parent

Original Name : Heidi Armbruster

Gender : Female

Character Name : Toy Store Parent

Original Name : Finnerty Steeves

Gender : Female

Character Name : Parent with Girls

Original Name : John Speredakos

Gender : Male

Character Name : Kicking Girl

Original Name : Skai Jackson

Gender : Female

Character Name : Skateboard Kid

Original Name : Alex Hall

Gender : Male

Character Name : Skateboard Kid

Original Name : Eric Redgate

Gender : Male

Character Name : FAO Custodian

Original Name : Jojo Gonzalez

Gender : Male

Character Name : Cop

Original Name : Scott Dillin

Gender : Male

Character Name : Cop

Original Name : Tyree Michael Simpson

Gender : Male

Character Name : Inmate Bubba

Original Name : Sean Ringgold

Gender : Male

Character Name : Bubba's Inmate Friend

Original Name : Mario D'Leon

Gender : Male

Character Name : Party Guest

Original Name : Liz Smith

Gender : Female

Character Name : Party Guest

Original Name : Tom Colicchio

Gender : Male

Character Name : Party Guest

Original Name : Michael Musto

Gender : Male

Character Name : Party Guest

Original Name : Joan Rivers

Gender : Female

Character Name : Party Guest

Original Name : Olivia Palermo

Gender : Female

Character Name : Party Guest

Original Name : Julia Enescu

Gender : Male

Character Name : Party Guest

Original Name : Lauren Waggoner

Gender : Male

Character Name : Azrael

Original Name : Mr. Krinkle

Gender : Male

Character Name : Elway

Original Name : Hank

Gender : Male

Character Name : Gutsy Smurf (voice)

Original Name : Alan Cumming

Gender : Male

Character Name : Brainy Smurf (voice)

Original Name : Fred Armisen

Gender : Male

Character Name : Grouchy Smurf (voice)

Original Name : George Lopez

Gender : Male

Character Name : Greedy Smurf (voice)

Original Name : Kenan Thompson

Gender : Male

Character Name : Handy Smurf (voice)

Original Name : Jeff Foxworthy

Gender : Male

Character Name : Vanity Smurf (voice)

Original Name : John Oliver

Gender : Male

Character Name : Chef Smurf (voice)

Original Name : Wolfgang Puck

Gender : Male

Character Name : Hefty Smurf (voice)

Original Name : Gary Basaraba

Gender : Male

Character Name : Jokey Smurf (voice)

Original Name : Paul Reubens

Gender : Male

Character Name : Baker Smurf (voice)

Original Name : B.J. Novak

Gender : Male

Character Name : Narrator Smurf (voice)

Original Name : Tom Kane

Gender : Male

Character Name : Crazy Smurf (Voice)

Original Name : John Kassir

Gender : Male

Character Name : Farmer Smurf (voice)

Original Name : Joel McCrary

Gender : Male

Character Name : Mother of Girl in Store (uncredited)

Original Name : Mary McGloin

Gender : Female